Synthesis and opioid activity of dynorphin A-(1-13)NH2 analogues containing cis- and trans-4-aminocyclohexanecarboxylic acid

J Med Chem. 1993 Apr 16;36(8):1100-3. doi: 10.1021/jm00060a018.

Abstract

It has been proposed that the "message" sequence of dynorphin A (Dyn A) exists in an extended conformation in aqueous solution (Schiller, P. W. Int. J. Pept. Protein Res. 1983, 21, 307-312). Molecular modeling suggested that trans-4-aminocyclohexanecarboxylic acid (trans-ACCA) might function as a conformationally constrained replacement for Gly2-Gly3 of Dyn A in such an extended conformation. ACCA was synthesized by catalytic hydrogenation of p-aminobenzoic acid, and the cis and trans isomers were separated by fractional recrystallization. Analogues of Dyn A-(1-13)-NH2 containing cis- and trans-ACCA were prepared by solid-phase peptide synthesis using the Fmoc chemical protocol. Results from radioligand binding assays indicated that the peptides have modest affinity for kappa opioid receptors (Ki's = 9.1 and 13.4 nM for [cis-ACCA2-3]- and [trans-ACCA2-3]Dyn A-(1-13)NH2, respectively) and modest kappa-receptor selectivity (Ki ratio (kappa/mu/delta) = 1/13/210 and 1/21/103, respectively). [cis-ACCA2-3]- and [trans-ACCA2-3]Dyn A-(1-13)-NH2 are the first reported Dyn A analogues constrained in the "message" sequence that are selective for kappa receptors. The cis-ACCA analogue showed very weak opioid activity (IC50 = 4.0 microM) in the guinea pig ileum.

Publication types

  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Amino Acids / chemical synthesis*
  • Amino Acids / metabolism
  • Amino Acids / pharmacology
  • Animals
  • Binding Sites
  • Cyclohexanecarboxylic Acids / chemical synthesis*
  • Cyclohexanecarboxylic Acids / metabolism
  • Cyclohexanecarboxylic Acids / pharmacology
  • Dynorphins / pharmacology*
  • Guinea Pigs
  • Muscle, Smooth / drug effects
  • Muscle, Smooth / metabolism
  • Narcotics / chemical synthesis*
  • Narcotics / metabolism
  • Narcotics / pharmacology
  • Peptide Fragments / pharmacology
  • Rats
  • Receptors, Opioid, kappa / metabolism
  • Stereoisomerism
  • Structure-Activity Relationship

Substances

  • Amino Acids
  • Cyclohexanecarboxylic Acids
  • Narcotics
  • Peptide Fragments
  • Receptors, Opioid, kappa
  • dynorphin (1-13)
  • Dynorphins